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Ti含量对Nb-Si基超高温合金组织及相成分的影响
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西北工业大学凝固技术国家重点实验室

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TG146.4

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国家自然科学基金项目(面上项目,重点项目,重大项目)


EFFECTS OF Ti CONTENT ON THE MICROSTRUCTURE AND PHASE COMPOSITIONS OF Nb-Si BASED ULTRAHIGH TEMPERATURE ALLOY
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State Key Laboratory of Solidification Processing, Northwestern Polytechnical University

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    摘要:

    采用真空非自耗电弧熔炼的方法制备了Nb-Si基超高温合金,分析了Ti含量对合金组织及相成分的影响规律。结果表明,合金中Ti含量不仅影响初生(Nb,X)5Si3的晶型,而且对其尺寸及含量也有明显影响。当加入的Ti含量较低时(0-10 at.%),初生硅化物为α-(Nb,X)5Si3;与未添加Ti的合金相比,含Ti合金的硅化物含量明显增加;当合金中加入的Ti含量为18-20 at.%时,初生硅化物为α-(Nb,X)5Si3和γ-(Nb,X)5Si3,但α-(Nb,X)5Si3的含量随着合金中Ti含量的增加而减少;当合金中加入的Ti含量为22-30 at.%时,初生硅化物仅为γ-(Nb,X)5Si3。随合金中Ti含量的增加,α-(Nb,X)5Si3的尺寸增大,但γ-(Nb,X)5Si3尺寸基本不变。Ti在Nbss和γ-(Nb,X)5Si3中的含量均随合金中Ti含量的增加而增加,但Ti在α-(Nb,X)5Si3中的含量较低且基本不随合金中Ti含量的增加而变化。Ti主要取代各相中的Nb,而对Al, Cr, Hf元素在各相中固溶倾向性的影响不明显。

    Abstract:

    Nb-Si based ultrahigh temperature alloys were prepared by vacuum non-consumable arc melting and the effects of Ti addition contents on their microstructure and phase composition were investigated. The results showed that Ti addition contents could exert an obvious influence on the types, sizes and area fractions of primary (Nb,X)5Si3 in the microstructure. When Ti addition content was relatively low (0-10 at.%), the primary silicides were α-(Nb,X)5Si3 and its area fraction increased significantly with increase in Ti addition content. When the Ti addition content was ranged from 18-20 at.%, the primary silicides were of two types: respectively α-(Nb,X)5Si3 and γ-(Nb,X)5Si3. However, the amount of α-(Nb,X)5Si3 decreased with increase in the Ti addition content in the alloy. When Ti addition content in the alloy varied from 22-30 at.%, there was only one form of primary silicides i.e., γ-(Nb,X)5Si3 left. Moreover, as the Ti addition content in the alloy increased, the size of α-(Nb,X)5Si3 increased while the size of γ-(Nb,X)5Si3 was less affected. In addition, as the Ti addition content in the alloy increased, Ti concentration in both Nbss and γ-(Nb,X)5Si3 increased while that in α-(Nb,X)5Si3 was lower and did not change obviously. It should also be noticed that Ti atoms only replaced Nb atoms in various phases while had no obvious effects on the solution tendency of other alloying elements such as Al, Cr and Hf.

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王高举,郭喜平. Ti含量对Nb-Si基超高温合金组织及相成分的影响[J].稀有金属材料与工程,2016,45(2):387~392.[wang gao ju, guo xiping. EFFECTS OF Ti CONTENT ON THE MICROSTRUCTURE AND PHASE COMPOSITIONS OF Nb-Si BASED ULTRAHIGH TEMPERATURE ALLOY[J]. Rare Metal Materials and Engineering,2016,45(2):387~392.]
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  • 收稿日期:2014-03-24
  • 最后修改日期:2014-07-31
  • 录用日期:2014-09-28
  • 在线发布日期: 2016-07-19
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