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Basic Thermodynamic Research of Eutectic High Entropy Alloy Formation
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National University of Defense Technology

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    Abstract:

    In this paper, by collecting and summarizing the reported overall composition and phase composition of 18 eutectic high-entropy alloys (EHEAs), some parameters reflecting their properties were calculated, including mixing enthalpy, mixing entropy, Gibbs free energy, atomic size mismatch, the electronegativity difference and the valence electron concentration , and the influence of these parameters on the structure of the alloy were analyzed from a thermodynamic point of view. It is found that the calculated mixed entropy equivalent of the overall composition of the eutectic high-entropy alloy basically meets the structural criterion requirements of the traditional high-entropy alloy to form a single-phase solid solution. (Such as △Smix >11 J/(mol·K)、-15 kJ/mol < △Hmix < 5 kJ/mol、δ < 6.6%) But because the average free energy of the eutectic phase is lower than the total free energy when the whole forms a single phase, this makes the eutectic high-entropy alloy in the solidification process A eutectic reaction occurs, forming a multi-phase structure.

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[Li Yahao, Tang Yu, Ye Yicong, Li Shun, Wan Hong, Liu Xiyue, Zhu Li’an, Wang Zhen, Bai Shuxin. Basic Thermodynamic Research of Eutectic High Entropy Alloy Formation[J]. Rare Metal Materials and Engineering,2021,50(5):1635~1640.]
DOI:10.12442/j. issn.1002-185X.20200474

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History
  • Received:July 04,2020
  • Revised:July 17,2020
  • Adopted:August 05,2020
  • Online: June 09,2021
  • Published: May 25,2021