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First-principles study on oxidation performance of TD3 alloy
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Taiyuan University of Technology

Clc Number:

TG146.2+3

Fund Project:

Supported by the Natural Science Foundation of Shanxi Province (Project No. 201801D121098), Youth Natural Science of Shanxi Province (201801D221339)

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    Abstract:

    The first-principles calculation method is used to study the alloy atom vacancy formation energies of O phase, B2 phase and α2 phase in TD3 alloy, and the energy stability and diffusion behavior of oxygen atoms in the three phases. The calculation results show that the vacancy formation energies of Al atoms in the three phases are all lower than those of Ti and Nb, which is beneficial to the formation of α-Al2O3 dominated oxide film on the surface of TD3 alloy. The interstitial energy of oxygen atoms in the octahedral interstitial positions of O phase, B2 phase and α2 phase is lower than that of tetrahedral interstitial positions, and the interstitial energy of titanium-rich octahedral interstitial positions is the lowest, the lowest oxygen atom interstitial energy is -5.0815eV respectively , -4.9425eV and -5.9315eV. The barriers to be crossed for oxygen atoms to diffuse along the best diffusion path in O phase, B2 phase and α2 phase are 0.812 eV, 1.913 eV and 1.164 eV, respectively.

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[He Longbin, Wang Wenbo, Zhang Jianlin, Wang Xudong, Duan Xinglu, Liu Qiuzu, Li Xiuyan. First-principles study on oxidation performance of TD3 alloy[J]. Rare Metal Materials and Engineering,2022,51(11):4237~4242.]
DOI:10.12442/j. issn.1002-185X.20210905

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History
  • Received:October 18,2021
  • Revised:January 06,2022
  • Adopted:January 29,2022
  • Online: December 02,2022
  • Published: November 30,2022