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Crystal structure and electrochemical performance of La0.6Sr0.4Co0.2Fe0.8-xScxO3-? cathode materials for solid oxide fuel cell
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TM911.4 ??????????????

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国家自然科学基金项目(51974167);内蒙古自治区高等学校创新团队发展计划支持(No.NMGIRT2215)

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    Abstract:

    The Sc-doped La0.6Sr0.4Co0.2Fe0.8-XScxO3-? (LSCFScx, x=0, 0.04, 0.08) cathode powders were synthesized by a sol-gel method. The crystal structure, chemical morphology of surface elements, catalytic activity and electrochemical properties of LSCFSc cathode material were systematically analyzed.XRD results show that LSCF has a cubic structure, and the LSCFSc cathode material changes from cubic to hexagonal structure.The conductivity of LSCFSc cathode material decreases with the Sc3+-doping, and the conductivity of LSCFSc0.08 cathode sample is still greater than 100 S/cm in the temperature range of 300-800.XPS results show that Sc3+-doping increases the content of adsorbed oxygen (OAds) on the surface of LSCFSc cathode material, and the RASR of polarization surface of LSCFSc0.08 cathode material measured at 800℃ is 0.026 Ω·cm2, which is about 87.6% lower than RASR of LSCF cathode material, which significantly improved the adsorption/dissociation ability of LSCFSc cathode material to oxygen, and enhanced the catalytic activity of oxygen.Ni-SDC as the anode material, SDC as electrolyte, and LSCFSc0.08 as cathode material assembled into Ni-SDC|SDC|LSCFSc0.08 anode-support single cell, the maximum power density is 806 mW/cm2 at 800 ℃, indicating that Sc3+-doping can significantly improved the electrochemical performance of cathode materials.

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[caichangkun, xiemanyi, wanglin, xueke, pengjun, baojinxiao, anshengli. Crystal structure and electrochemical performance of La0.6Sr0.4Co0.2Fe0.8-xScxO3-? cathode materials for solid oxide fuel cell[J]. Rare Metal Materials and Engineering,2023,52(2):601~608.]
DOI:10.12442/j. issn.1002-185X.20220008

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History
  • Received:January 05,2022
  • Revised:March 06,2022
  • Adopted:March 28,2022
  • Online: March 09,2023
  • Published: February 28,2023